LrgpV1, Main, Exploration, bibRecord, 000423

Development of a CO2 Capture Process Based on Ammonia Solvent and a Dedicated Composite Hollow Fibre Membrane Contactor

Identifieur interne : 000423 ( Main/Exploration ); précédent : 000422; suivant : 000424

Development of a CO2 Capture Process Based on Ammonia Solvent and a Dedicated Composite Hollow Fibre Membrane Contactor

Auteurs : Yann Le Moullec [France] ; Thibaut Neveux [France] ; Kamel Makhloufi [France] ; Denis Roizard [France] ; Mohamed Kanniche [France] ; Éric Favre (génie des procédés) [France]

Source :

RBID : Hal:hal-01276055

Abstract

CO2 capture is recognized as necessary to achieve significant greenhouse gas emission reduction before 2050. Regarding these technologies, the main issue is the high cost of avoided CO2 related to capture (approximate to 40 (sic)/t). In conventional amine-based CO2 capture process, the four main key parameters driving the cost of avoided CO2 are the regeneration duty, the compression works, the compressor cost and the solvent make-up cost. On the one hand, the use of hollow fibre membrane contactor (HFMC) for CO2 capture is foreseen to be an efficient technology for absorber intensification; but regarding the impact of the absorber cost on the cost of avoided CO2, the use of HFMC for process intensification does not seem relevant. On the other hand, ammonia as solvent for CO2 capture is a cheap solvent with no degradation problem. Moreover, it allows a high pressure regeneration reducing the compression works. The key idea of this work is to find a membrane with high CO2/NH3 selectivity and high permeability in order to use aqueous ammonia as a solvent in a HFMC in order to reduce significantly the ammonia slip in flue gases while maintaining high absorption rate. The work has been divided in three main steps: the screening of available material for the membrane, the laboratory test of the membrane and the modelling of the system for process assessment. For this absorption device a total equivalent work of 240 kWh/ t(CO2) has been calculated for CO2 capture on a coal-fired power plant.

Url:

https://hal.univ-lorraine.fr/hal-01276055

DOI: 10.1016/j.egypro.2014.11.072

Affiliations:

Links toward previous steps (curation, corpus...)

to stream Hal, to step Corpus: 000326
to stream Hal, to step Curation: 000326
to stream Hal, to step Checkpoint: 000433
to stream Main, to step Merge: 000440
to stream Main, to step Curation: 000423

Le document en format XML

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<orgName>Université de Lorraine</orgName>
<orgName type="acronym">UL</orgName>
<date type="start">2012-01-01</date>
<desc><address><addrLine>34 cours Léopold - CS 25233 - 54052 Nancy cedex</addrLine>
<country key="FR"></country>
</address>
<ref type="url">http://www.univ-lorraine.fr/</ref>
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<idno type="IdRef">02636817X</idno>
<orgName>Centre National de la Recherche Scientifique</orgName>
<orgName type="acronym">CNRS</orgName>
<date type="start">1939-10-19</date>
<desc><address><country key="FR"></country>
</address>
<ref type="url">http://www.cnrs.fr/</ref>
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<country>France</country>
<placeName><settlement type="city">Nancy</settlement>
<settlement type="city">Metz</settlement>
<region type="region" nuts="2">Grand Est</region>
<region type="old region" nuts="2">Lorraine (région)</region>
</placeName>
<orgName type="university">Université de Lorraine</orgName>
<placeName><settlement type="city">Nancy</settlement>
<region type="region" nuts="2">Grand Est</region>
<region type="region" nuts="2">Lorraine (région)</region>
</placeName>
<orgName type="laboratoire" n="5">Laboratoire réactions et génie des procédés</orgName>
<orgName type="university">Université de Lorraine</orgName>
<orgName type="institution">Centre national de la recherche scientifique</orgName>
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<idno type="DOI">10.1016/j.egypro.2014.11.072</idno>
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<front><div type="abstract" xml:lang="en">CO2 capture is recognized as necessary to achieve significant greenhouse gas emission reduction before 2050. Regarding these technologies, the main issue is the high cost of avoided CO2 related to capture (approximate to 40 (sic)/t). In conventional amine-based CO2 capture process, the four main key parameters driving the cost of avoided CO2 are the regeneration duty, the compression works, the compressor cost and the solvent make-up cost. On the one hand, the use of hollow fibre membrane contactor (HFMC) for CO2 capture is foreseen to be an efficient technology for absorber intensification; but regarding the impact of the absorber cost on the cost of avoided CO2, the use of HFMC for process intensification does not seem relevant. On the other hand, ammonia as solvent for CO2 capture is a cheap solvent with no degradation problem. Moreover, it allows a high pressure regeneration reducing the compression works. The key idea of this work is to find a membrane with high CO2/NH3 selectivity and high permeability in order to use aqueous ammonia as a solvent in a HFMC in order to reduce significantly the ammonia slip in flue gases while maintaining high absorption rate. The work has been divided in three main steps: the screening of available material for the membrane, the laboratory test of the membrane and the modelling of the system for process assessment. For this absorption device a total equivalent work of 240 kWh/ t(CO2) has been calculated for CO2 capture on a coal-fired power plant.</div>
</front>
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<affiliations><list><country><li>France</li>
</country>
<region><li>Grand Est</li>
<li>Lorraine (région)</li>
</region>
<settlement><li>Metz</li>
<li>Nancy</li>
</settlement>
<orgName><li>Centre national de la recherche scientifique</li>
<li>Laboratoire réactions et génie des procédés</li>
<li>Université de Lorraine</li>
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<tree><country name="France"><noRegion><name sortKey="Le Moullec, Yann" sort="Le Moullec, Yann" uniqKey="Le Moullec Y" first="Yann" last="Le Moullec">Yann Le Moullec</name>
</noRegion>
<name sortKey="Favre, Eric" sort="Favre, Eric" uniqKey="Favre E" first="Eric" last="Favre">Éric Favre (génie des procédés)</name>
<name sortKey="Kanniche, Mohamed" sort="Kanniche, Mohamed" uniqKey="Kanniche M" first="Mohamed" last="Kanniche">Mohamed Kanniche</name>
<name sortKey="Makhloufi, Kamel" sort="Makhloufi, Kamel" uniqKey="Makhloufi K" first="Kamel" last="Makhloufi">Kamel Makhloufi</name>
<name sortKey="Neveux, Thibaut" sort="Neveux, Thibaut" uniqKey="Neveux T" first="Thibaut" last="Neveux">Thibaut Neveux</name>
<name sortKey="Roizard, Denis" sort="Roizard, Denis" uniqKey="Roizard D" first="Denis" last="Roizard">Denis Roizard</name>
</country>
</tree>
</affiliations>
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Development of a CO2 Capture Process Based on Ammonia Solvent and a Dedicated Composite Hollow Fibre Membrane Contactor

Development of a CO2 Capture Process Based on Ammonia Solvent and a Dedicated Composite Hollow Fibre Membrane Contactor

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